Ratchet-induced variations in bulk states of an active ideal gas

Publication date

2018-11-07

Authors

Rodenburg, Anne JeroenISNI 0000000493281007
Paliwal, SiddharthISNI 0000000506036589
De Jager, Marjolein
Bolhuis, Peter G.
Dijkstra, MarjoleinISNI 0000000358257928
Roij, René vanISNI 0000000392993654

Editors

Advisors

Supervisors

Document Type

Article
Open Access logo

License

Abstract

We study the distribution of active, noninteracting particles over two bulk states separated by a ratchet potential. By solving the steady-state Smoluchowski equations in a flux-free setting, we show that the ratchet potential affects the distribution of particles over the bulks and thus exerts an influence of infinitely long range. As we show, an external potential that is nonlinear is crucial for having such a long-range influence. We characterize how the difference in bulk densities depends on activity and on the ratchet potential, and we identify power law dependencies on system parameters in several limiting cases. While weakly active systems are often understood in terms of an effective temperature, we present an analytical solution that explicitly shows that this is not possible in the current setting. Instead, we rationalize our results by a simple transition state model that presumes particles to cross the potential barrier by Arrhenius rates modified for activity. While this model does not quantitatively describe the difference in bulk densities for feasible parameter values, it does reproduce - in its regime of applicability - the complete power law behavior correctly.

Keywords

Taverne, General Physics and Astronomy, Physical and Theoretical Chemistry

Citation

Rodenburg, J, Paliwal, S, De Jager, M, Bolhuis, P G, Dijkstra, M & Van Roij, R 2018, 'Ratchet-induced variations in bulk states of an active ideal gas', Journal of Chemical Physics, vol. 149, no. 17, 174910. https://doi.org/10.1063/1.5048698