Suppression of Carbon Deposition in the Iron-Catalyzed Production of Lower Olefins from Synthesis Gas
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Publication date
2012
Authors
Koeken, Ard C J
Torres Galvis, H.M.
Davidian, T.
Ruitenbeek, M.
de Jong, K.P.
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Abstract
A tapered-element oscillating microbalance was used to evaluate carbon deposition on a highly selective and active supported iron catalyst for the production of lower olefins. With increasing pressure, the H2/CO ratio had a profound effect on the carbon deposition rate and accordingly, conditions leading to minimal carbon deposition, low methane selectivity, and high olefin selectivity were identified.
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Koeken, A C J, Torres Galvis, H M, Davidian, T, Ruitenbeek, M & de Jong, K P 2012, 'Suppression of Carbon Deposition in the Iron-Catalyzed Production of Lower Olefins from Synthesis Gas', Angewandte Chemie-International Edition, vol. 51, no. 29, pp. 7190-7193. https://doi.org/10.1002/anie.201200280