Increasing the Lipophilic Character of Tetraphenylborate Anions through Silyl Substituents

Publication date

2001

Authors

Koten, G. van
Broeke, J. van den
Lutz, M.H.
Kooijman, H.
Spek, A.L.
Deelman, B.J.

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Abstract

Trimethylsilyl- and dimethyl(1H,1H,2H,2H-perfluorooctyl)silyl substituents have been introduced in the para position of tetraphenylborate anions, resulting in enhanced solubility of their complexes n-Bu4N[B(C6H4SiMe2R-4)4] (R = Me, CH2CH2C6F13) and [Rh(dppe)2][B(C6H4SiMe2R-4)4] (dppe = 1,2-bis(diphenylphosphino)ethane, R = Me, CH2CH2C6F13) in apolar organic solvents.

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